Wednesday, November 14, 2012

1211.2813 (C. -C. Chen et al.)

Doping Evolution of Oxygen K-edge X-ray Absorption Spectra in Cuprate
Superconductors
   [PDF]

C. -C. Chen, M. Sentef, Y. F. Kung, C. J. Jia, R. Thomale, B. Moritz, A. P. Kampf, T. P. Devereaux
We study oxygen K-edge x-ray absorption spectroscopy (XAS) and investigate the validity of the Zhang-Rice singlet (ZRS) picture in overdoped cuprate superconductors. Using large-scale exact diagonalization of the three-orbital Hubbard model, we observe the effect of strong correlations manifesting in a dynamical spectral weight transfer from the upper Hubbard band to the ZRS band. The quantitative agreement between theory and experiment highlights an additional spectral weight reshuffling due to core-hole interaction. Our results confirm the important correlated nature of the cuprates and elucidate the changing orbital character of the low-energy quasi-particles, but also demonstrate the continued relevance of the ZRS even in the overdoped region.
View original: http://arxiv.org/abs/1211.2813

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